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Reversible Photoswitching in Poly(2-oxazoline) Nanoreactors

Chemistry. 2020-04-01; 
Michael Kuepfert, Peiyuan Qu, Aaron Cohen, Caroline Hoyt, Christopher Jones, Marcus Weck
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Codon Optimization … accession numbers AAA25265 and NP_999039, respectively. DNA sequences encoding for these two proteins were purchased from Genscript with codons optimized for E. coli expression. The G6PDH and cMDH genes were … Get A Quote

摘要

This contribution reports light responsive catalytic nanoreactors based on poly(2-oxazoline) diblock copolymers. The hydrophobic block of the copolymer is a random copolymer consisting of a spiropyran functionalized 2-oxazoline (SPOx) and 2-(but-3-yn-1-yl)-4,5-dihydrooxazole (ButynOx), while the hydrophilic block is based on 2-methyl-2-oxazoline (MeOx). The block copolymer is terminated with tris(2-aminoethyl) amine (TREN) that serves as catalyst in a Knoevenagel condensation. Four block copolymers with different ButynOx/SPOx and hydrophilic/hydrophobic ratios are synthesized and self-assembled through solvent exchange. Micelles and vesicles of various sizes are observed by TEM, which undergo morphological and ... More

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